Which Chip are you using?
change line 61 from
#define DATA_TRANSFER_MODE TLC_SPI
to
#define DATA_TRANSFER_MODE TLC_BITBANG
Then look at lines 73-79
Change them from
/** SIN (TLC pin 26) */
#define SIN_PIN DEFAULT_BB_SIN_PIN
#define SIN_PORT DEFAULT_BB_SIN_PORT
#define SIN_DDR DEFAULT_BB_SIN_DDR
/** SCLK (TLC pin 25) */
#define SCLK_PIN DEFAULT_BB_SCLK_PIN
#define SCLK_PORT DEFAULT_BB_SCLK_PORT
#define SCLK_DDR DEFAULT_BB_SCLK_DDR
to
/** SIN (TLC pin 26) */
#define SIN_PIN PD5
#define SIN_PORT PORTD
#define SIN_DDR DDRD
/** SCLK (TLC pin 25) */
#define SCLK_PIN PD6
#define SCLK_PORT PORTD
#define SCLK_DDR DDRD
That will use pins 4 and 5 on the arduino I am assuming you are using an UNO (ATMega168)