What kind of changes do I have to make in this library's FreqCountTimers.h or other files for Attiny3226 (Megatinycore)?
I also use the TCA0 timer to generate bit PWM on the same processor. Do I have problems with PWM or frequency counting?
After a quick glance in the source I think the hardware dependent coding is all in the UTIL subdirectory. You would have to add the timer definitions for the Attiny3226 (family) there and give it a try.
Maybe easier to program TCB yourself as it supports Input Capture Frequency Measurement.